A general method to synthesize and sinter bulk ceramics in seconds

Chengwei Wang(University of Maryland, College Park), Weiwei Ping(University of Maryland, College Park), Qiang Bai(University of Maryland, College Park), Huachen Cui(University of California, Los Angeles), Ryan Hensleigh(University of California, Los Angeles), Ruiliu Wang(University of Maryland, College Park), Alexandra H. Brozena(University of Maryland, College Park), Zhenpeng Xu(University of California, Los Angeles), Jiaqi Dai(University of Maryland, College Park), Yong Pei(University of Maryland, College Park), Chaolun Zheng(University of Maryland, College Park), Glenn Pastel(University of Maryland, College Park), Jinlong Gao(University of Maryland, College Park), Xizheng Wang(University of Maryland, College Park), Howard Wang(University of Maryland, College Park), Ji‐Cheng Zhao(University of Maryland, College Park), Bao Yang(University of Maryland, College Park), Xiaoyu Zheng(University of California, Los Angeles), Jian Luo(University of California San Diego), Yifei Mo(University of Maryland, College Park), Bruce Dunn(University of California, Los Angeles), Liangbing Hu(University of Maryland, College Park)
Science
April 30, 2020
Cited by 755Open Access
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Abstract

Ceramics are an important class of materials with widespread applications because of their high thermal, mechanical, and chemical stability. Computational predictions based on first principles methods can be a valuable tool in accelerating materials discovery to develop improved ceramics. It is essential to experimentally confirm the material properties of such predictions. However, materials screening rates are limited by the long processing times and the poor compositional control from volatile element loss in conventional ceramic sintering techniques. To overcome these limitations, we developed an ultrafast high-temperature sintering (UHS) process for the fabrication of ceramic materials by radiative heating under an inert atmosphere. We provide several examples of the UHS process to demonstrate its potential utility and applications, including advancements in solid-state electrolytes, multicomponent structures, and high-throughput materials screening.


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