Enhancement of Single-Molecule Fluorescence Using a Gold Nanoparticle as an Optical NanoantennaSergei Kühn, Ulf Håkanson, L. Rogobete et al.|Physical Review Letters|2006 We investigate the coupling of a single molecule to a single spherical gold nanoparticle acting as a nanoantenna. Using scanning probe technology, we position the particle in front of the molecule with nanometer accuracy and measure a strong enhancement of more than 20 times in the fluorescence intensity simultaneous to a 20-fold shortening of the excited state lifetime. Comparisons with three-dimensional calculations guide us to decipher the contributions of the excitation enhancement, spontaneous emission modification, and quenching. Furthermore, we provide direct evidence for the role of the particle plasmon resonance in the molecular excitation and emission processes.
Detection and Spectroscopy of Gold Nanoparticles Using Supercontinuum White Light Confocal MicroscopyWe combine confocal microscopy using supercontinuum laser illumination and an interferometric detection technique to identify single nanoparticles of diameter below 10 nm. Spectral analysis of the signal allows us to record the plasmon resonance of a single nanoparticle. Our results hold great promise for fundamental studies of the optical properties of single metal clusters and for their use in biophysical applications.
Very low threshold whispering-gallery-mode microsphere laserWe report on the realization of a whispering-gallery-mode laser based on neodymium-doped silica microspheres. Absorbed pump powers at threshold are as low as 200 nW. The linear variation of the threshold with the loss factor of the cavity mode has also been observed. We discuss the potential of this system as a permanent microlaser operating with a few active ions at liquid-helium temperature.
Measurement of the Casimir-Polder forceC. I. Sukenik, M. G. Boshier, D. Cho et al.|Physical Review Letters|1993 We have studied the deflection of ground-state sodium atoms passing through a micron-sized parallel-plate cavity by measuring the intensity of a sodium atomic beam transmitted through the cavity as a function of cavity plate separation. This experiment provides clear evidence for the existence of the Casimir-Polder force, which is due to modification of the ground-state Lamb shift in the confined space of a cavity. Our results confirm the magnitude of the force and the distance dependence predicted by quantum electrodynamics.
Direct printing of nanostructures by electrostatic autofocussing of ink nanodroplets