Magnesium- and intermetallic alloys-based hydrides for energy storage: modelling, synthesis and properties

Luca Pasquini(University of Bologna), Kouji Sakaki(National Institute of Advanced Industrial Science and Technology), Etsuo Akiba(Kyushu University), Mark D. Allendorf(Sandia National Laboratories California), Ebert Alvares(Helmholtz-Zentrum Hereon), J.R. Ares(Universidad Autónoma de Madrid), Dotan Babai(Ben-Gurion University of the Negev), Marcello Baricco(National Interuniversity Consortium of Materials Science and Technology), José M. Bellosta von Colbe(Helmholtz-Zentrum Hereon), M. Bereznitsky(Ben-Gurion University of the Negev), Craig E. Buckley(Curtin University), Young Whan Cho(Korea Institute of Science and Technology), Fermín Cuevas(Centre National de la Recherche Scientifique), Patricia de Rango(Centre National de la Recherche Scientifique), Erika Michela Dematteis(National Interuniversity Consortium of Materials Science and Technology), R.V. Denys(Institute for Energy Technology), Martin Dornheim(Helmholtz-Zentrum Hereon), J.F. Fernandez(Universidad Autónoma de Madrid), Arif Hariyadi(Sepuluh Nopember Institute of Technology), Bjørn C. Hauback(Institute for Energy Technology), Tae Wook Heo(Lawrence Livermore National Laboratory), Michael Hirscher(Max Planck Institute for Intelligent Systems), Terry D. Humphries(Curtin University), Jacques Huot(Université du Québec à Trois-Rivières), I. Jacob(Ben-Gurion University of the Negev), Torben R. Jensen(Aarhus University), Paul Jerabek(Helmholtz-Zentrum Hereon), ShinYoung Kang(Lawrence Livermore National Laboratory), Nathan Keilbart(Lawrence Livermore National Laboratory), Hyunjeong Kim(National Institute of Advanced Industrial Science and Technology), M. Latroche(Centre National de la Recherche Scientifique), Fabrice Leardini(Universidad Autónoma de Madrid), Haiwen Li(Hefei General Machinery Research Institute (China)), Sanliang Ling(University of Nottingham), Mykhaylo Lototskyy(University of the Western Cape), Ryan Gotchy Mullen(Lawrence Livermore National Laboratory), Shin‐ichi Orimo(Tohoku University), Mark Paskevicius(Curtin University), Claudio Pistidda(Helmholtz-Zentrum Hereon), Marek Polański(Military University of Technology in Warsaw), Julián Puszkiel(Helmut Schmidt University), Eugen Rabkin(Technion – Israel Institute of Technology), Martin Sahlberg(Uppsala University), Sabrina Sartori(University of Oslo), Archa Santhosh(Helmholtz-Zentrum Hereon), Toyoto Sato(Shibaura Institute of Technology), Roni Z. Shneck(Ben-Gurion University of the Negev), Magnus H. Sørby(Institute for Energy Technology), Yuanyuan Shang(Helmholtz-Zentrum Hereon), Vitalie Stavila(Sandia National Laboratories California), Jin‐Yoo Suh(Korea Institute of Science and Technology), Suwarno Suwarno(Sepuluh Nopember Institute of Technology), Le Thi Thu(Helmholtz-Zentrum Hereon), Liwen F. Wan(Lawrence Livermore National Laboratory), C. J. Webb(Griffith University), Matthew Witman(Sandia National Laboratories California), Chubin Wan(University of Science and Technology Beijing), Brandon C. Wood(Lawrence Livermore National Laboratory), V.A. Yartys(Institute for Energy Technology)
Progress in Energy
June 8, 2022
10.1088/2516-1083/ac7190
Cited by 122Open Access
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Abstract

Abstract Hydrides based on magnesium and intermetallic compounds provide a viable solution to the challenge of energy storage from renewable sources, thanks to their ability to absorb and desorb hydrogen in a reversible way with a proper tuning of pressure and temperature conditions. Therefore, they are expected to play an important role in the clean energy transition and in the deployment of hydrogen as an efficient energy vector. This review, by experts of Task 40 ‘Energy Storage and Conversion based on Hydrogen’ of the Hydrogen Technology Collaboration Programme of the International Energy Agency, reports on the latest activities of the working group ‘Magnesium- and Intermetallic alloys-based Hydrides for Energy Storage’. The following topics are covered by the review: multiscale modelling of hydrides and hydrogen sorption mechanisms; synthesis and processing techniques; catalysts for hydrogen sorption in Mg; Mg-based nanostructures and new compounds; hydrides based on intermetallic TiFe alloys, high entropy alloys, Laves phases, and Pd-containing alloys. Finally, an outlook is presented on current worldwide investments and future research directions for hydrogen-based energy storage.

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