Hydrogen storage in complex hydrides: past activities and new trends

Erika Michela Dematteis(National Interuniversity Consortium of Materials Science and Technology), Mads B. Amdisen(Aarhus University), Tom Autrey(Pacific Northwest National Laboratory), Jussara Barale(National Interuniversity Consortium of Materials Science and Technology), Mark Bowden(Pacific Northwest National Laboratory), Craig E. Buckley(Curtin University), Young Whan Cho(Korea Institute of Science and Technology), Stefano Deledda(Institute for Energy Technology), Martin Dornheim(Helmholtz-Zentrum Hereon), Petra E. de Jongh(Utrecht University), Jakob B. Grinderslev(Aarhus University), Gökhan Gizer(Helmholtz-Zentrum Hereon), Valerio Gulino(Utrecht University), Bjørn C. Hauback(Institute for Energy Technology), Michael Heere(Technische Universität Braunschweig), Tae Wook Heo(Lawrence Livermore National Laboratory), Terry D. Humphries(Curtin University), Torben R. Jensen(Aarhus University), ShinYoung Kang(Lawrence Livermore National Laboratory), Young‐Su Lee(Korea Institute of Science and Technology), Haiwen Li(Hefei General Machinery Research Institute (China)), Sichi Li(Lawrence Livermore National Laboratory), Kasper T. Møller(Aarhus University), Peter Ngene(Utrecht University), Shin‐ichi Orimo(Tohoku University), Mark Paskevicius(Curtin University), Marek Polański(Military University of Technology in Warsaw), Shigeyuki Takagi(Tohoku University), Liwen F. Wan(Lawrence Livermore National Laboratory), Brandon C. Wood(Lawrence Livermore National Laboratory), Michael Hirscher(Max Planck Institute for Intelligent Systems), Marcello Baricco(National Interuniversity Consortium of Materials Science and Technology)
Progress in Energy
May 30, 2022
10.1088/2516-1083/ac7499
Cited by 102Open Access
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Abstract

Abstract Intense literature and research efforts have focussed on the exploration of complex hydrides for energy storage applications over the past decades. A focus was dedicated to the determination of their thermodynamic and hydrogen storage properties, due to their high gravimetric and volumetric hydrogen storage capacities, but their application has been limited because of harsh working conditions for reversible hydrogen release and uptake. The present review aims at appraising the recent advances on different complex hydride systems, coming from the proficient collaborative activities in the past years from the research groups led by the experts of the Task 40 ‘Energy Storage and Conversion Based on Hydrogen’ of the Hydrogen Technology Collaboration Programme of the International Energy Agency. An overview of materials design, synthesis, tailoring and modelling approaches, hydrogen release and uptake mechanisms and thermodynamic aspects are reviewed to define new trends and suggest new possible applications for these highly tuneable materials.

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