Phosphine–imine and –enamido ligands for acceptorless dehydrogenation catalysis

James M. Stubbs(Western University), Kelly F. Firth(Western University), Benjamin J. Bridge(Western University), Kathleen J. Berger(Western University), Richard J. Hazlehurst(Western University), P. D. Boyle(Western University), Johanna M. Blacquiere(Western University)
Dalton Transactions
November 28, 2016
Cited by 11Open Access
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Abstract

A highly tunable phosphine-imine ligand family is introduced. Following metallation with ruthenium, deprotonation of the ligand affords a phosphine-enamido species. Complexes with the ligand in both the imine and enamido forms are active toward acceptorless dehydrogenation reactions.


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