Metal‐Free Aminosulfonylation of Aryldiazonium Tetrafluoroborates with DABCO⋅(SO<sub>2</sub>)<sub>2</sub> and Hydrazines

Danqing Zheng(Fudan University), Yuanyuan An(Fudan University), Zhen Hua Li(Fudan University), Jie Wu(Chinese Academy of Sciences)
Angewandte Chemie International Edition
January 29, 2014
Cited by 288

Abstract

The coupling of aryldiazonium tetrafluoroborates, DABCO⋅(SO2)2, and hydrazines under metal-free conditions leads to the formation of aryl N-aminosulfonamides. The reaction proceeds smoothly at room temperature and shows broad functional-group tolerance. A radical process is proposed for this transformation.


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