The Influence of Hydrogen‐Bond Defects on the Properties of Ionic Liquids
Tim Peppel(University of Rostock), Christian Roth(University of Rostock), Koichi Fumino(University of Rostock), Dietmar Paschek(University of Rostock), Martin Köckerling(University of Rostock), Ralf Ludwig(University of Rostock)
Cited by 136
Abstract
Counterintuitive: The preformation of ion pairs can explain the low melting points of imidazolium-based ionic liquids (ILs) and the resulting expanded range of working temperatures. This quasi-ion-pair formation is possible for ILs having cations with only one interaction site leading to local and directional hydrogen bonds with the corresponding anion (see structure; O red, N blue, F green, S yellow).
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