Solar hydrogen production with semiconductor metal oxides: new directions in experiment and theory
Álvaro Valdés(Consejo Superior de Investigaciones Científicas), Jérémie Brillet(École Polytechnique Fédérale de Lausanne), Michaël Grätzel(École Polytechnique Fédérale de Lausanne), Hildur Gudmundsdóttir(University of Iceland), Heine Anton Hansen(Technical University of Denmark), Hannes Jónsson(SLAC National Accelerator Laboratory), P. Klüpfel(University of Iceland), Geert–Jan Kroes(Leiden University), Florian Le Formal(École Polytechnique Fédérale de Lausanne), Isabela C. Man(Technical University of Denmark), Rafael S. Martins(Chalmers University of Technology), Jens K. Nørskov(SLAC National Accelerator Laboratory), Jan Rossmeisl(Technical University of Denmark), Kevin Sivula(École Polytechnique Fédérale de Lausanne), Aleksandra Vojvodić(Stanford University), Michael Zäch(Chalmers University of Technology)
Cited by 217Open Access
Abstract
An overview of a collaborative experimental and theoretical effort toward efficient hydrogen production via photoelectrochemical splitting of water into di-hydrogen and di-oxygen is presented here. We present state-of-the-art experimental studies using hematite and TiO(2) functionalized with gold nanoparticles as photoanode materials, and theoretical studies on electro and photo-catalysis of water on a range of metal oxide semiconductor materials, including recently developed implementation of self-interaction corrected energy functionals.
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