Neutron Scattering from a Liquid on a Jump Diffusion Model

Abstract

The incoherent inelastic scattering cross section of slow neutrons from liquids is calculated using a simple model in which the liquid is assumed to have appreciable short range order in a quasi-crystalline form. Diffusive motion takes place in large discrete jumps, between which the atoms oscillate as in a solid. The model predicts a definite, easily calculable cross section which is not dominated by diffusion effects as when continuous diffusion is assumed, but shows a characteristic variation with angle which could be looked for experimentally. The related pair correlation functions are dominated at small r and t by vibrational effects. Although simple and extreme the model explains several aspects of the observations of Brockhouse and Pope in 1959 and others. A brief discussion of the coherent scattering cross sections for the model is given although explicit formulae are not obtained.